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Tytuł:
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Ultrafast Interfacial Self-Assembly of 2D Transition Metal Dichalcogenides Monolayer Films and Their Vertical and In-Plane Heterostructures.
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Autorzy:
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Yun T; National Creative Research Initiative Center for Multi-Dimensional Directed Nanoscale Assembly, Department of Materials Science and Engineering, KAIST , Daejeon 34141, Republic of Korea.
Kim JS; Department of Chemical and Biomolecular Engineering, KAIST , Daejeon 34141, Republic of Korea.
Shim J; AMOREPACIFIC Co. R&D Center , Yongin, 446-729, Republic of Korea.
Choi DS; National Creative Research Initiative Center for Multi-Dimensional Directed Nanoscale Assembly, Department of Materials Science and Engineering, KAIST , Daejeon 34141, Republic of Korea.
Lee KE; National Creative Research Initiative Center for Multi-Dimensional Directed Nanoscale Assembly, Department of Materials Science and Engineering, KAIST , Daejeon 34141, Republic of Korea.
Koo SH; National Creative Research Initiative Center for Multi-Dimensional Directed Nanoscale Assembly, Department of Materials Science and Engineering, KAIST , Daejeon 34141, Republic of Korea.
Kim I; National Creative Research Initiative Center for Multi-Dimensional Directed Nanoscale Assembly, Department of Materials Science and Engineering, KAIST , Daejeon 34141, Republic of Korea.
Jung HJ; National Creative Research Initiative Center for Multi-Dimensional Directed Nanoscale Assembly, Department of Materials Science and Engineering, KAIST , Daejeon 34141, Republic of Korea.
Yoo HW; Department of Chemical and Biomolecular Engineering, KAIST , Daejeon 34141, Republic of Korea.
Jung HT; Department of Chemical and Biomolecular Engineering, KAIST , Daejeon 34141, Republic of Korea.
Kim SO; National Creative Research Initiative Center for Multi-Dimensional Directed Nanoscale Assembly, Department of Materials Science and Engineering, KAIST , Daejeon 34141, Republic of Korea.
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Źródło:
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ACS applied materials & interfaces [ACS Appl Mater Interfaces] 2017 Jan 11; Vol. 9 (1), pp. 1021-1028. Date of Electronic Publication: 2016 Dec 28.
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Typ publikacji:
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Journal Article
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Język:
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English
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Imprint Name(s):
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Original Publication: Washington, D.C. : American Chemical Society
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Contributed Indexing:
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Keywords: assembly; film; interface; sensor; transition metal dichalcogenide
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Entry Date(s):
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Date Created: 20161215 Date Completed: 20180727 Latest Revision: 20180727
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Update Code:
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20240105
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DOI:
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10.1021/acsami.6b11365
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PMID:
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27966907
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Cost effective scalable method for uniform film formation is highly demanded for the emerging applications of 2D transition metal dichalcogenides (TMDs). We demonstrate a reliable and fast interfacial self-assembly of TMD thin films and their heterostructures. Large-area 2D TMD monolayer films are assembled at air-water interface in a few minutes by simple addition of ethyl acetate (EA) onto dilute aqueous dispersions of TMDs. Assembled TMD films can be directly transferred onto arbitrary nonplanar and flexible substrates. Precise thickness controllability of TMD thin films, which is essential for thickness-dependent applications, can be readily obtained by the number of film stacking. Most importantly, complex structures such as laterally assembled 2D heterostructures of TMDs can be assembled from mixture solution dispersions of two or more different TMDs. This unusually fast interfacial self-assembly could open up a novel applications of 2D TMD materials with precise tunability of layer number and film structures.