Nanoscale Chemical Imaging of Zeolites Using Atom Probe Tomography.

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Abstrakt

Tytuł:: Nanoscale Chemical Imaging of Zeolites Using Atom Probe Tomography.
Autorzy:: Schmidt JE; Debye Institute for Nanomaterials Science, Utrecht University, Universiteitsweg 99, 3584, CG, Utrecht, The Netherlands.
Peng L; Grinnell College, 1115 8th Ave, Grinnell, IA, 50112, USA.
Poplawsky JD; Center for Nanophase Materials Sciences, Oak Ridge National Laboratory, Oak Ridge, TN 37831-6064, USA.
Weckhuysen BM; Debye Institute for Nanomaterials Science, Utrecht University, Universiteitsweg 99, 3584, CG, Utrecht, The Netherlands.
Źródło:: Angewandte Chemie (International ed. in English) [Angew Chem Int Ed Engl] 2018 Aug 13; Vol. 57 (33), pp. 10422-10435. Date of Electronic Publication: 2018 Jul 24.
Typ publikacji:: Journal Article; Review
Język:: English
Imprint Name(s):: Publication: <2004-> : Weinheim : Wiley-VCH
Original Publication: Weinheim/Bergstr. : New York, : Verlag Chemie ; Academic Press, c1962-
References:: Chem Soc Rev. 2010 Dec;39(12):4703-17. (PMID: 20953505)
Chem Soc Rev. 2010 Dec;39(12):4754-66. (PMID: 20981379)
Ultramicroscopy. 2015 Dec;159 Pt 2:324-37. (PMID: 26095825)
Nat Chem. 2012 Nov;4(11):873-86. (PMID: 23089861)
Ultramicroscopy. 2007 Sep;107(9):761-6. (PMID: 17403581)
Ultramicroscopy. 2014 Jun;141:16-21. (PMID: 24704605)
Ultramicroscopy. 2011 May;111(6):469-72. (PMID: 21664542)
Angew Chem Int Ed Engl. 2016 Sep 5;55(37):11173-7. (PMID: 27485276)
Ultramicroscopy. 2007 Feb-Mar;107(2-3):131-9. (PMID: 16938398)
Chem Soc Rev. 2010 Dec;39(12):5051-66. (PMID: 21038052)
Ultramicroscopy. 2009 Sep;109(10):1304-9. (PMID: 19592168)
Micron. 2015 Jan;68:146-151. (PMID: 24931385)
Chem Soc Rev. 2010 Dec;39(12):4783-93. (PMID: 21038051)
Nat Nanotechnol. 2011 May;6(5):302-7. (PMID: 21478867)
J Microsc. 2010 Feb;237(2):155-67. (PMID: 20096046)
Microsc Res Tech. 2008 Jul;71(7):542-50. (PMID: 18425800)
Chem Soc Rev. 2010 Dec;39(12):4626-42. (PMID: 20949188)
Ultramicroscopy. 2005 Mar;102(4):287-98. (PMID: 15694675)
Nature. 2011 Jan 13;469(7329):194-7. (PMID: 21228873)
MethodsX. 2014 Mar 05;1:12-8. (PMID: 26150928)
Chem Soc Rev. 2014 Feb 21;43(4):990-1006. (PMID: 24085063)
J Phys Chem Lett. 2013 Mar 21;4(6):993-8. (PMID: 26291366)
Angew Chem Int Ed Engl. 2018 Aug 13;57(33):10422-10435. (PMID: 29718553)
Chem Soc Rev. 2015 Oct 21;44(20):7234-61. (PMID: 26007224)
Chem Soc Rev. 2010 Dec;39(12):4951-5001. (PMID: 21038053)
Microsc Microanal. 2010 Feb;16(1):99-110. (PMID: 20082732)
Microscopy (Oxf). 2013 Feb;62(1):109-46. (PMID: 23349242)
Microsc Microanal. 2013 Jun;19(3):652-64. (PMID: 23668837)
Science. 2017 Sep 1;357(6354):898-903. (PMID: 28818971)
Chem Soc Rev. 2010 Dec;39(12):4560-70. (PMID: 20886166)
J Microsc. 2001 Sep;203(Pt 3):295-302. (PMID: 11555147)
Ultramicroscopy. 2015 Dec;159 Pt 2:420-6. (PMID: 25748692)
Rev Sci Instrum. 2007 Mar;78(3):031101. (PMID: 17411171)
Nat Mater. 2008 Dec;7(12):992-6. (PMID: 18997774)
Angew Chem Int Ed Engl. 2009;48(27):4910-43. (PMID: 19536746)
Chemphyschem. 2010 Apr 6;11(5):951-62. (PMID: 20306509)
Ultramicroscopy. 2003 Sep;96(3-4):433-51. (PMID: 12871806)
Nano Lett. 2014 Aug 13;14(8):4220-3. (PMID: 24989063)
Nat Commun. 2015 Jul 02;6:7589. (PMID: 26133270)
J Microsc. 2004 Dec;216(Pt 3):234-40. (PMID: 15566495)
ChemCatChem. 2017 Jan 9;9(1):17-29. (PMID: 28239429)
Chem Soc Rev. 2015 Oct 21;44(20):7022-4. (PMID: 26401967)
Nat Commun. 2017 Nov 21;8(1):1666. (PMID: 29162802)
Nature. 2013 Apr 4;496(7443):78-82. (PMID: 23552946)
J Phys Chem Lett. 2014 Apr 17;5(8):1361-7. (PMID: 26269980)
Science. 2007 Apr 27;316(5824):561-5. (PMID: 17463280)
Ultramicroscopy. 2015 Dec;159 Pt 2:413-9. (PMID: 25980894)
Ultramicroscopy. 2004 Jul;100(1-2):25-34. (PMID: 15219690)
Langmuir. 2012 Jan 24;28(3):1673-7. (PMID: 22220909)
Sci Rep. 2016 Nov 23;6:37586. (PMID: 27876869)
Ultramicroscopy. 2015 Dec;159 Pt 2:354-9. (PMID: 25796357)
Nat Commun. 2016 Jul 27;7:12537. (PMID: 27460872)
Nat Commun. 2015 Aug 14;6:8014. (PMID: 26272722)
Chem Soc Rev. 2010 Dec;39(12):4864-84. (PMID: 20972502)
Chem Soc Rev. 2010 Dec;39(12):4741-53. (PMID: 20978666)
Contributed Indexing:: Keywords: acidity; atom probe tomography; heterogeneous catalysis; single-atom microscopy; zeolites
Entry Date(s):: Date Created: 20180503 Latest Revision: 20210109
Update Code:: 20240104
PubMed Central ID:: PMC6519151
DOI:: 10.1002/anie.201712952
PMID:: 29718553
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Understanding structure-composition-property relationships in zeolite-based materials is critical to engineering improved solid catalysts. However, this can be difficult to realize as even single zeolite crystals can exhibit heterogeneities spanning several orders of magnitude, with consequences for, for example, reactivity, diffusion as well as stability. Great progress has been made in characterizing these porous solids using tomographic techniques, though each method has an ultimate spatial resolution limitation. Atom probe tomography (APT) is the only technique so far capable of producing 3D compositional reconstructions with sub-nanometer-scale resolution, and has only recently been applied to zeolite-based catalysts. Herein, we discuss the use of APT to study zeolites, including the critical aspects of sample preparation, data collection, assignment of mass spectral peaks including the predominant CO peak, the limitations of spatial resolution for the recovery of crystallographic information, and proper data analysis. All sections are illustrated with examples from recent literature, as well as previously unpublished data and analyses to demonstrate practical strategies to overcome potential pitfalls in applying APT to zeolites, thereby highlighting new insights gained from the APT method.
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