Triple-Responsive Polyampholytic Graft Copolymers as Smart Sensors with Varying Output.

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Tytuł:: Triple-Responsive Polyampholytic Graft Copolymers as Smart Sensors with Varying Output.
Autorzy:: Max JB; Institute of Organic Chemistry and Macromolecular Chemistry, Friedrich-Schiller-Universität Jena, Lessingstraße 8, Jena, 07743, Germany.; Jena Center for Soft Matter (JCSM), Friedrich-Schiller-Universität Jena, Philosophenweg 7, Jena, 07743, Germany.; Center for Energy and Environmental Chemistry (CEEC), Friedrich-Schiller-Universität Jena, Philosophenweg 7, Jena, 07743, Germany.
Nabiyan A; Institute of Organic Chemistry and Macromolecular Chemistry, Friedrich-Schiller-Universität Jena, Lessingstraße 8, Jena, 07743, Germany.; Jena Center for Soft Matter (JCSM), Friedrich-Schiller-Universität Jena, Philosophenweg 7, Jena, 07743, Germany.; Center for Energy and Environmental Chemistry (CEEC), Friedrich-Schiller-Universität Jena, Philosophenweg 7, Jena, 07743, Germany.
Eichhorn J; Institute of Organic Chemistry and Macromolecular Chemistry, Friedrich-Schiller-Universität Jena, Lessingstraße 8, Jena, 07743, Germany.; Jena Center for Soft Matter (JCSM), Friedrich-Schiller-Universität Jena, Philosophenweg 7, Jena, 07743, Germany.; Center for Energy and Environmental Chemistry (CEEC), Friedrich-Schiller-Universität Jena, Philosophenweg 7, Jena, 07743, Germany.
Schacher FH; Institute of Organic Chemistry and Macromolecular Chemistry, Friedrich-Schiller-Universität Jena, Lessingstraße 8, Jena, 07743, Germany.; Jena Center for Soft Matter (JCSM), Friedrich-Schiller-Universität Jena, Philosophenweg 7, Jena, 07743, Germany.; Center for Energy and Environmental Chemistry (CEEC), Friedrich-Schiller-Universität Jena, Philosophenweg 7, Jena, 07743, Germany.
Źródło:: Macromolecular rapid communications [Macromol Rapid Commun] 2021 Apr; Vol. 42 (7), pp. e2000671. Date of Electronic Publication: 2020 Dec 28.
Typ publikacji:: Journal Article
Język:: English
Imprint Name(s):: Publication: 2002- : Weinheim, Germany : Wiley-VCH
Original Publication: Basel ; Oxford, CT : Hüthig & Wepf, c1994-
MeSH Terms:: Metal Nanoparticles*
Polymers ; Silver ; Surface Plasmon Resonance ; Temperature
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Grant Information:: SCHA1640/18-1 Deutsche Forschungsgemeinschaft
Contributed Indexing:: Keywords: graft copolymers; metal sensors; polyampholyte; smart polymers; stimuli responsive materials
Substance Nomenclature:: 0 (Polymers)
3M4G523W1G (Silver)
Entry Date(s):: Date Created: 20201228 Date Completed: 20210621 Latest Revision: 20210621
Update Code:: 20240105
DOI:: 10.1002/marc.202000671
PMID:: 33368771
: Czasopismo naukowe

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Three triggers result in two measurable outputs from polymeric sensors: multiresponsive polyampholytic graft copolymers respond to pH-value and temperature, as well as the type and concentration of metal cations and therefore, allow the transformation of external triggers into simply measurable outputs (cloud point temperature (T CP ) and surface plasmon resonance (SPR) of encapsulated silver nanoparticles). The synthesis relies on poly(dehydroalanine) (PDha) as the reactive backbone and gives straightforward access to materials with tunable composition and output. In particular, a rather high sensitivity toward the presence of Cu 2+ , Co 2+ , and Pb 2+ metal cations is found.
(© 2020 The Authors. Macromolecular Rapid Communications published by Wiley-VCH GmbH.)

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