Charge-Reversible Surfactant-Induced Transformation Between Oil-in-Dispersion Emulsions and Pickering Emulsions.

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Tytuł:: Charge-Reversible Surfactant-Induced Transformation Between Oil-in-Dispersion Emulsions and Pickering Emulsions.
Autorzy:: Jiang J; The Key Laboratory of Synthetic and Biological Colloids, Ministry of Education, School of Chemical and Material Engineering, Jiangnan University, 1800 Lihu Road, Wuxi, Jiangsu, 214122, China.
Yu S; The Key Laboratory of Synthetic and Biological Colloids, Ministry of Education, School of Chemical and Material Engineering, Jiangnan University, 1800 Lihu Road, Wuxi, Jiangsu, 214122, China.
Zhang W; The Key Laboratory of Synthetic and Biological Colloids, Ministry of Education, School of Chemical and Material Engineering, Jiangnan University, 1800 Lihu Road, Wuxi, Jiangsu, 214122, China.
Zhang H; The Key Laboratory of Synthetic and Biological Colloids, Ministry of Education, School of Chemical and Material Engineering, Jiangnan University, 1800 Lihu Road, Wuxi, Jiangsu, 214122, China.
Cui Z; The Key Laboratory of Synthetic and Biological Colloids, Ministry of Education, School of Chemical and Material Engineering, Jiangnan University, 1800 Lihu Road, Wuxi, Jiangsu, 214122, China.
Xia W; State Key Laboratory of Food Science and Technology, School of Food Science and Technology, Jiangnan University, 1800 Lihu Road, Wuxi, Jiangsu, 214122, China.
Binks BP; Department of Chemistry, University of Hull, Hull, HU6 7RX, UK.
Źródło:: Angewandte Chemie (International ed. in English) [Angew Chem Int Ed Engl] 2021 May 17; Vol. 60 (21), pp. 11793-11798. Date of Electronic Publication: 2021 Apr 16.
Typ publikacji:: Journal Article
Język:: English
Imprint Name(s):: Publication: <2004-> : Weinheim : Wiley-VCH
Original Publication: Weinheim/Bergstr. : New York, : Verlag Chemie ; Academic Press, c1962-
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Contributed Indexing:: Keywords: Pickering emulsion; charge-reversible; silica nanoparticles; surfactant
Entry Date(s):: Date Created: 20210319 Latest Revision: 20210511
Update Code:: 20240105
DOI:: 10.1002/anie.202102098
PMID:: 33739584
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A novel charge-reversible surfactant, (CH 3 ) 2 N-(CH 2 ) 10 COONa, was designed and synthesized, which together with silica nanoparticles can stabilize a smart n-octane-in-water emulsion responsive to pH. At high pH (9.3) the surfactant is anionic carboxylate, which together with the negatively charged silica nanoparticles co-stabilize flowable oil-in-dispersion emulsions, whereas at low pH (4.1) it is turned to cationic form by forming amine salt which can hydrophobize in situ the negatively charged silica nanoparticles to stabilize viscous oil-in-water (O/W) Pickering emulsions. At neutral pH (7.5), however, this surfactant is converted to zwitterionic form, which only weakly hydrophobises the silica particles to stabilize O/W Pickering emulsions of large droplet size. Moreover, demulsification can be achieved rapidly triggered by pH. With this strategy particles can be controlled either dispersed in water or adsorbed at the oil-water interface endowing emulsions with the capacity for intelligent and precise control of stability as well as viscosity and droplet size.
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