Porous Carbon Architecture Assembled by Cross-Linked Carbon Leaves with Implanted Atomic Cobalt for High-Performance Li-S Batteries.

Tytuł:: Porous Carbon Architecture Assembled by Cross-Linked Carbon Leaves with Implanted Atomic Cobalt for High-Performance Li-S Batteries.
Autorzy:: Wang R; Department of Materials Science, Fudan University, Shanghai, 200433, People's Republic of China.
Wu R; Department of Materials Science, Fudan University, Shanghai, 200433, People's Republic of China. .
Ding C; Department of Materials Science, Fudan University, Shanghai, 200433, People's Republic of China.
Chen Z; Department of Materials Science, Fudan University, Shanghai, 200433, People's Republic of China.
Xu H; Department of Materials Science, Fudan University, Shanghai, 200433, People's Republic of China.
Liu Y; State Key Laboratory of Silicon Materials and School of Materials Science and Engineering, Zhejiang University, Hangzhou, 310027, People's Republic of China. .
Zhang J; Shanghai Synchrotron Radiation Facility, Zhangjiang Laboratory, Shanghai Advanced Research Institute, Chinese Academy of Sciences, Shanghai, 201204, People's Republic of China.
Ha Y; Department of Materials Science, Fudan University, Shanghai, 200433, People's Republic of China.
Fei B; Department of Materials Science, Fudan University, Shanghai, 200433, People's Republic of China.
Pan H; State Key Laboratory of Silicon Materials and School of Materials Science and Engineering, Zhejiang University, Hangzhou, 310027, People's Republic of China. .; Institute of Science and Technology for New Energy, Xi'an Technological University, Xi'an, 710021, People's Republic of China. .
Źródło:: Nano-micro letters [Nanomicro Lett] 2021 Jun 30; Vol. 13 (1), pp. 151. Date of Electronic Publication: 2021 Jun 30.
Typ publikacji:: Journal Article
Język:: English
Imprint Name(s):: Publication: [Berlin] : Springer
Original Publication: Fayetteville, Ark. : OAHOST
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Contributed Indexing:: Keywords: 3D porous carbon architecture; Cathode; Lithium–sulfur battery; Single-atom Co
Entry Date(s):: Date Created: 20210701 Latest Revision: 20220831
Update Code:: 20240105
PubMed Central ID:: PMC8245650
DOI:: 10.1007/s40820-021-00676-6
PMID:: 34195913
: Czasopismo naukowe

Pełny tekst

The practical application of lithium-sulfur batteries is severely hampered by the poor conductivity, polysulfide shuttle effect and sluggish reaction kinetics of sulfur cathodes. Herein, a hierarchically porous three-dimension (3D) carbon architecture assembled by cross-linked carbon leaves with implanted atomic Co-N 4 has been delicately developed as an advanced sulfur host through a SiO 2 -mediated zeolitic imidazolate framework-L (ZIF-L) strategy. The unique 3D architectures not only provide a highly conductive network for fast electron transfer and buffer the volume change upon lithiation-delithiation process but also endow rich interface with full exposure of Co-N 4 active sites to boost the lithium polysulfides adsorption and conversion. Owing to the accelerated kinetics and suppressed shuttle effect, the as-prepared sulfur cathode exhibits a superior electrochemical performance with a high reversible specific capacity of 695 mAh g -1 at 5 C and a low capacity fading rate of 0.053% per cycle over 500 cycles at 1 C. This work may provide a promising solution for the design of an advanced sulfur-based cathode toward high-performance Li-S batteries.

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