Bio-Based, Recyclable and Self-Healing Polyurethane Composites with High Energy Dissipation and Shape Memory.

Szczegóły
Abstrakt

Tytuł:: Bio-Based, Recyclable and Self-Healing Polyurethane Composites with High Energy Dissipation and Shape Memory.
Autorzy:: Shou T; State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing, 100029, China.; Beijing Engineering Research Center of Advanced Elastomers, Beijing University of Chemical Technology, Beijing, 100029, China.
Zhai M; State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing, 100029, China.; Beijing Engineering Research Center of Advanced Elastomers, Beijing University of Chemical Technology, Beijing, 100029, China.
Wu Y; State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing, 100029, China.; Beijing Engineering Research Center of Advanced Elastomers, Beijing University of Chemical Technology, Beijing, 100029, China.
Wu S; State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing, 100029, China.; Key Laboratory of Carbon Fiber and Functional Polymers, Ministry of Education, Beijing University of Chemical Technology, Beijing, 10029, China.; Beijing Engineering Research Center of Advanced Elastomers, Beijing University of Chemical Technology, Beijing, 100029, China.
Hu S; State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing, 100029, China.; Key Laboratory of Carbon Fiber and Functional Polymers, Ministry of Education, Beijing University of Chemical Technology, Beijing, 10029, China.; Beijing Engineering Research Center of Advanced Elastomers, Beijing University of Chemical Technology, Beijing, 100029, China.
Zhao X; State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing, 100029, China.; Key Laboratory of Carbon Fiber and Functional Polymers, Ministry of Education, Beijing University of Chemical Technology, Beijing, 10029, China.; Beijing Engineering Research Center of Advanced Elastomers, Beijing University of Chemical Technology, Beijing, 100029, China.
Zhang L; State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing, 100029, China.; Key Laboratory of Carbon Fiber and Functional Polymers, Ministry of Education, Beijing University of Chemical Technology, Beijing, 10029, China.; Beijing Engineering Research Center of Advanced Elastomers, Beijing University of Chemical Technology, Beijing, 100029, China.
Źródło:: Macromolecular rapid communications [Macromol Rapid Commun] 2022 Nov; Vol. 43 (21), pp. e2200486. Date of Electronic Publication: 2022 Sep 16.
Typ publikacji:: Journal Article
Język:: English
Imprint Name(s):: Publication: 2002- : Weinheim, Germany : Wiley-VCH
Original Publication: Basel ; Oxford, CT : Hüthig & Wepf, c1994-
MeSH Terms:: Polyurethanes*/chemistry
Polyesters*/chemistry
Humans ; Tensile Strength ; Temperature ; Viscosity
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Grant Information:: 51988102 National Natural Science Foundation of China; 52203003 National Science Foundation for Young Scientists of China
Contributed Indexing:: Keywords: energy dissipation; polylactic acid; polyurethane; self-healing; shape memory
Substance Nomenclature:: 0 (Polyurethanes)
0 (Polyesters)
Entry Date(s):: Date Created: 20220810 Date Completed: 20221107 Latest Revision: 20221107
Update Code:: 20240105
DOI:: 10.1002/marc.202200486
PMID:: 35947533
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Rubber composites make an important contribution to eliminating vibration and noise owing to their unique viscoelasticity. However, it is important to find alternative bio-based products with high damping properties owing to the shortage of petrochemical resources and poor performance. The ability to self-heal is an additional characteristic that is highly desirable because it can further increase the service life and safety of such products. In this study, a bio-based polylactic acid thermoplastic polyurethane (PLA-TPU) and its composites (PLA-TPU/AO-80) are synthesized. The reversible sacrificial hydrogen bonds in the composites increase the peak value of the loss factor (tan δ max ) from 0.87 to 2.12 with a high energy dissipation efficiency of 99% at 50% strain. After being heated for 15 min, the healed sample recovers 81.98% of its comprehensive mechanical properties due to the reorganization of the hydrogen bonds. Its tensile strength remains at 93.4% after recycling five times. Moreover, its shape memory properties show a response temperature close to the human body temperature making it an ideal candidate for medical applications.
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